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Tuning Brønsted Acidity by up to 12 pKa Units in a Redox-Active Nanopore Lined with Multifunctional Metal Sites

By Taro Jones and others
Electrostatic interactions, hydrogen bonding, and solvation effects can alter the free energies of ionizable functional groups in proteins and other enclosed porous architectures, allowing these nanostructures to tune acid-base chemistry as needed to support specific functions. Herein, we expand on this theme to examine how metal sites (M = H2,... Show more
June 26, 2024
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Tuning Brønsted Acidity by up to 12 pKa Units in a Redox-Active Nanopore Lined with Multifunctional Metal Sites
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